Ps. Banks et al., High-intensity third-harmonic generation in beta barium borate through second-order and third-order susceptibilities, OPTICS LETT, 24(1), 1999, pp. 4-6
The azimuthal dependence of third-order and cascaded second-order nonlinear
coupling was used to measure the relative contributions of each to direct
third-harmonic generation in beta-barium berate. This permitted the measure
ment of the values of tensor elements chi(10)((3)), chi(11)((3)), and chi(1
6)((3)) relative to the known chi(ij)((2)). Finally, conversion efficiencie
s to 3 omega of up to 6% were achieved with a femtosecond chirped-pulse amp
lification laser with 200 GW/cm(2) in collimated beams. (C) 1999 Optical So
ciety of America.