The real dielectric constant epsilon' and loss factor tan delta were s
tudied as function of frequency f, temperature T and composition x for
a series of samples of BaCo2x ZnxFe12-2xO19 hexagonal ferrite system
with x = 0.4, 0.8, 1.2, 1.6 and 2 prepared using the usual ceramic tec
hnique. The experimental results indicated that epsilon' and tan delta
decrease as the frequency increases and temperature decreases. The st
udied samples showed abnormal dielectric behavior (or relaxation peaks
) which were shifted towards higher frequency as the temperature and s
ubstitution of Co and Zn ions increase. Increasing the Co and Zn ions
substitution for x I 1.2, epsilon' and tan delta decrease reaching min
ima while activation energy for dielectric relaxation ED and pre-expon
ential constant f(0) increase reaching maxima at x = 1.2. The behavior
was reversed for x > 1.2, where epsilon' and tan delta increase while
E-D and f(0) decrease.