The Microwave Limb Sounder (MLS) experiments obtain measurements of atmosph
eric composition, temperature, and pressure by observations of millimeter-
and submillimeter-wavelength thermal emission as the instrument field of vi
ew is scanned through the atmospheric limb. Features of the measurement tec
hnique include the ability to measure many atmospheric gases as well as tem
perature and pressure, to obtain measurements even in the presence of dense
aerosol and cirrus, and to provide near-global coverage on a daily basis a
t all times of day and night from an orbiting platform. The composition mea
surements are relatively insensitive to uncertainties in atmospheric temper
ature. An accurate spectroscopic database is available, and the instrument
calibration is also very accurate and stable. The first MLS experiment in s
pace, launched on the (NASA) Upper Atmosphere Research Satellite (UARS) in
September 1991, was designed primarily to measure stratospheric profiles of
ClO, O-3, H2O, and atmospheric pressure as a vertical reference. Global me
asurement of ClO, the predominant radical in chlorine destruction of ozone,
was an especially important objective of UARS MLS. Ail objectives of UARS
MLS have been accomplished and additional geophysical products beyond those
for which the experiment was designed have been obtained, including measur
ement of upper-tropospheric water vapor, which is important for climate cha
nge studies. A follow-on MLS experiment is being developed for NASA's Earth
Observing System (EOS) and is scheduled to be launched on the EOS CHEMISTR
Y platform in late 2002. EOS MLS is designed for many stratospheric measure
ments, including HO, radicals, which could not be measured by UARS because
adequate technology was not available, and better and more extensive upper-
tropospheric and lower-stratospheric measurements.