Gas phase C-60 is resonantly excited using picosecond infrared (IR) pulses
from a free electron laser. The excitation can be very high, reaching level
s where the thermal emission of electrons from C-60 is observed. The excita
tion is much more efficient when the IR radiation is chirped to lower frequ
encies during the excitation process. The excitation process is modeled and
the results are compared to the experiment. (C) 1998 Optical Society of Am
erica.