Structure and magnetism of pulsed-laser-deposited ultrathin films of Fe onCu(100)

A layer-by-layer growth of ultrathin films right from the beginning would b e desirable for establishing a straightforward correlation between magnetis m and structure. We give experimental evidence that with the help of pulsed laser deposition (PLD) we can achieve layer-by-layer growth for Fe on Cu(1 00) in contrast to deposition by molecular-beam epitaxy. We present the res ults of a comprehensive study of the structural and magnetic properties of PLD-grown ultrathin Fe films of thicknesses between 2 and 10 monolayers (ML ) deposited at room temperature. We show scanning tunneling microscopy imag es and low-energy electron-diffraction (LEED) patterns as well as intensity vs energy (IV) LEED curves demonstrating that PLD-grown Fe/Cu(100) has an isotropic fee structure. We characterize the magnetic properties of our fil ms by the magnetooptical Ken effect. Following the improved growth and morp hology, we found strong differences in the magnetic behavior of these films in comparison with Fe thermally deposited onto Cu(100): PLD-grown ultrathi n Fe/Cu(100) shows an in-plane easy axis of magnetization in the thickness range 2-5 ML and again from about 10 ML. where the film structure is domina ted by the bcc-Fe bulk phase, while there is a perpendicular easy axis of m agnetization between 7 and 10 ML coverage. These results are discussed in t erms of the different growth and structure due to the characteristic featur es of the PLD technique. [S0163-1829(99)13201-6].