Ripening suppression and large photoluminescence blueshift in aligned InGaAs quantum dots on a vicinal, (100) GaAs substrate

We observe ripening suppression in aligned InGaAs quantum dots (QDs) along multiatomic steps on a vicinal (100) GaAs substrate. By varying the growth interruption times, a study of QD morphologies by atomic force microscope r eveals a clear Ostwald ripening suppression effect on QD formation. On the other hand, we observe a regular ripening for InGaAs QDs on an exact (100) substrate. In addition, n-QD chains aligned along multiatomic steps are obs erved. An inhomogeneously broadened photoluminescence (PL) spectrum with la rger spectral width is obtained for a QD ensemble on a vicinal (100) substr ate as compared to those on an exact (100) substrate although statistical a nalyses of QD size distributions show similar size dispersions. The spectra l broadening is attributed to the lateral quantum coupling of aligned n-QD chains. PL spectra for QDs on vicinal (100) substrates show a larger rate o f blueshift with increasing interruption times, which is interpreted as a l ack of the PL compensation effect by size enlargement of the QDs during gro wth interruption. Thus the result supports the ripening suppression effect which is observed in the morphology study. (C) 1999 American Institute of P hysics. [S0021-8979(99)10503-6].