A comparison of 3D static light-scattering experiments with Monte Carlo simulations

The problems arising in conventional static light-scattering experiments wi th turbid samples due to multiple scattering of light can be overcome by th e cross correlation technique. We recently reported results of 3D cross cor relation experiments in which the angle dependence of the experimentally de termined values of the singly scattered light intensity agrees with that of the scattering cross section of the suspended particles. In this paper we present measurements for various optical path lengths of the scattered ligh t and compare the experimental results with Monte Carlo simulations. We dem onstrate that the dependences of the singly and multiply scattered light in tensities on the optical path length obtained by the 3D cross correlation m ethod are in good agreement with the data obtained from Monte Carlo simulat ions. These results further confirm that the 3D cross correlation technique indeed allows the direct determination of the singly scattered light inten sity by experimental means without any need for the detailed information ab out the experimental set-up that is necessary in Monte Carlo simulations.