A mode-locked titanium sapphire laser, tuneable over the region from 680 nm
to 1000 nm, has been used to generate monochromatic laser radiation over t
he region from 250 nm to 450 nm by second and third harmonic generation, wi
th power outputs of between 50 mW and 200 mW above 350 nm and around 30 mW
between 250 nm and 300 nm. The (pulsed) radiation was assessed as follows f
or its suitability as a source for the calibration of detectors in continuo
us-wave (cw) applications. (i) Radiation at 356.41 nm was used to calibrate
a trap detector for spectral responsivity against the National Physical La
boratory (NPL) cryogenic radiometer, and this value was compared with the o
ne obtained using a cw laser at the same wavelength: the values differed by
0.06%. (ii) The linearity of response of the trap detector was determined
at 362.0 nm. It was found to be linear to within 0.01% for powers up to 1.5
mW. The laser was then used to calibrate a trap detector for spectral resp
onsivity against the cryogenic radiometer over the region from 350 nm to 36
0 nm, with an estimated standard uncertainty of less than 0.1%.