Transition temperature between phase I (paramagnetic phase) and II (antifer
ro-quadrupolar ordered phase), T-Q, in magnetic fields up to 15 T is invest
igated for a high-quality single-crystal Ce0.4La0.6B6 by specific heat meas
urements. For H(0 0 1) T-Q increases with magnetic field up to similar to 1
2 T, as is known for larger x. However, T-Q shows a decrease with magnetic
held above similar to 12 T, which indicates that phase II closes in the H-T
plane, While in H(1 1 0) T-Q continues to increase with magnetic field up
to similar to 15 T and remarkable anisotropy of the phase boundary in the h
igh-held region is revealed. (C) 1999 Elsevier Science B.V. All rights rese
rved.