SHAPING MOLECULAR-BEAMS WITH INTENSE LIGHT

Authors
Citation
T. Seideman, SHAPING MOLECULAR-BEAMS WITH INTENSE LIGHT, The Journal of chemical physics, 107(24), 1997, pp. 10420-10429
Citations number
40
ISSN journal
00219606
Volume
107
Issue
24
Year of publication
1997
Pages
10420 - 10429
Database
ISI
SICI code
0021-9606(1997)107:24<10420:SMWIL>2.0.ZU;2-D
Abstract
We discuss the possibility of manipulating the center-of-mass motion o f molecules using the nonlinear interaction of a moderately intense, l ong-pulse laser field with the molecular polarizability tenser. Recent theoretical work demonstrating the possibility of focusing and trappi ng molecules is extended to consider the effects of circularly and ell iptically polarized light and the effect of nonspherical laser optics. The aberrations affecting the quality of the ''molecular lens'' are a nalyzed and the means by which they can be minimized are discussed. Mo lecular focusing is extended to a general field of molecular optics; t he possibilities of steering, reflecting, and collimating molecular be ams are illustrated. Application of the mechanical force of light to d isperse and separate species according to their mass, velocity, or qua ntum state is proposed. (C) 1997 American Institute of Physics.