The magnetization of rare-earth superlattices of Eu/Se grown on BaF2(1
1 1) by means of Molecular Beam Epitaxy (MBE) method has been measure
d in order to clarify the mechanism for the anomalous magnetic propert
ies. Selenium layers in the Eu/Se superlattice act as a separator betw
een Eu layers and the thickness of Se layers was varied from 0.5 to 3
nm, while that of Eu layers was fixed at 1 nm. The crystal structure o
f samples was characterized by X-ray diffraction and the in situ RHEED
observations. A considerably good epitaxial structure was attained fo
r [Eu 1 nm/Se 1 nm] sample, but [Eu 1 nm/Se 0.5 nm] and [Eu 1 nm/Se 3
nm] samples were only polycrystalline. The magnetization process measu
red at 1.9 K shows that a magnetic phase transition takes place from a
n antiferromagnetic to a spin-flop state. The critical magnetic field
H-C is obtained at 3750, 2150 and 1000 G, respectively, for [Eu 1 nm/S
e 0.5 nm], [Eu 1 nm/Se 1 nm] and [Eu 1 nm/Se 3 nm] samples. The exchan
ge integral J is dependent on the distance between Eu-Eu layers, i.e.,
J proportional to d(-1.1). The magnetic phase diagram of Eu/Se superl
attice has been obtained. (C) 1997 Elsevier Science Ltd.