By means of the on-line mass separator at Gesellschaft fur Schwerionen
forschung, Darmstadt, we produced Ba-114 through the Ni-51(Ni-58,2n) r
eaction, separated it as a (BaF+)-Ba-114-F-19 beam, and implanted it i
nto a stopper foil positioned in the center of an array of track detec
tors, which were used to search for C-12 radioactivity of Ba-114. A to
tal number of (5.4+/-1.7)X10(4 114)Ba atoms were implanted. No C-12 ev
ent was found after a total exposure time of 116 h, corresponding to a
Ni-58 beam dose of 1.3X10(17). The resulting upper limit of 3.4x10(-5
) (84% C.L.) for the branching ratio for C-12 decay of Ba-114 is consi
derably lower than the limits obtained in previous experiments, which
represents an inconsistency at levels of more than 90%. A semiempirica
l estimate of 19.3 MeV for the upper limit of the Q value for C-12 dec
ay of Ba-114 is derived.