S. Lupi et al., FANO EFFECT IN THE A-B PLANE OF ND1.96CE0.04CUO4- EVIDENCE OF PHONON INTERACTION WITH A POLARONIC BACKGROUND(Y ), Physical review. B, Condensed matter, 57(2), 1998, pp. 1248-1252
Reflectance measurements in different Nd1.96Ce0.04CuO4+y samples with
properly selected carrier concentrations provide firm evidence of Fano
antiresonances for the four transverse optical E-u phonons in the a-b
plane. An analysis of the Fano line shapes and of the dependence on t
emperature of the renormalized phonon frequencies allows us to determi
ne the origin of the electronic continuum interacting with the phonons
. Unlike in doped semiconductors. where the continuum is the free-carr
ier absorption band, here the continuum is provided by a polaron band
at similar to 0.1 eV, present in most parent compounds of high-T-c sup
erconductors. In the most doped sample, the polaron band softens as T
decreases, thus indicating a delocalization of the polaronic carriers
at low temperature.