Simultaneous, planar laser-induced fluorescence (LIF) images of nitric
oxide (NO) and acetone have been used to calculate instantaneous quan
titative maps of molecularly mixed jet-fluid fraction in an axisymmetr
ic shear layer. In this experiment, NO is seeded into high-purity nitr
ogen jet fluid and acetone is seeded into air coflow. On mixing at the
molecular level, the NO LIF is strongly quenched by oxygen from the c
oflow, while the acetone signal is unaffected by the mixing process. T
he extent to which the jet fluid is mixed at the molecular level is de
termined on a pixel-by-pixel basis from the simultaneous NO and aceton
e planar LIF images. Jets at Reynolds numbers ranging from 1000 to 50
000 are investigated. (C) 1997 Optical Society of America.