P. Jund et al., STRUCTURAL AND VIBRATIONAL PROPERTIES OF A SOFT-SPHERE GLASS - INFLUENCE OF THE QUENCHING RATE, Philosophical magazine. B. Physics of condensed matter.Statistical mechanics, electronic, optical and magnetic, 77(2), 1998, pp. 313-320
Using classical molecular dynamics simulations combined with the Voron
oi tessellation we study, at very low temperatures, the phonon spectru
m and the geometrical modifications in a model glass as a function of
the quenching rate. The shape of the phonon spectrum is not strongly a
ffected by a decrease in the quenching rate, except for the minimum pu
lsation omega(m), corresponding to the first pseudo-Bragg peak wave-ve
ctor, which goes through a marked minimum for the critical quenching r
ate at which the onset of crystallization is detected by the geometric
al analysis. This decrease in omega(m) can be interpreted as an increa
se in structural order in the glass phase when the cooling rate is low
ered.