We describe a study of samples grown by molecular-beam epitaxy, design
ed to examine the limitations to silicon (Si) delta-doping of gallium
arsenide (GaAs) at elevated growth temperatures. Samples (Si delta-dop
ed to 1 x 10(13) cm(-2)) were grown at 630 degrees C, during which the
growth was paused (for times between 0 and Is min) after depositing t
he Si. Total electron sheet densities were measured (using Hall and Sh
ubnikov-de Haas (SdH) effect measurements) to determine the electrical
ly active Si concentration. The free electron concentration showed a r
eduction from about 8 x 10(12) cm(-2) for zero pause time, to 5 x 10(1
2) cm(-2) for 18 min pause time. These results can be explained convin
cingly using simple models of impurity background in the MBE chamber o
r surface aggregation. Further experiments to distinguish these mechan
isms are discussed. (C) 1998 Elsevier Science B.V.