B. Barbara et al., QUANTUM RESONANCE OF THE MAGNETIZATION IN A SINGLE-CRYSTAL OF MN-12-AC, Journal of magnetism and magnetic materials, 177, 1998, pp. 1324-1329
In this study we raise a few questions regarding the hypothesis of con
servation of the collective spin in molecular crystals, some of them o
f interest for a deeper understanding of resonant tunnelling in Mn-12-
ac. We also show experimentally that in this system, resonant tunnelli
ng is not solely thermally activated, but takes place from the ground
state m = 10 below 2 K. The effects of a quartic anisotropy term on ma
gnetization curves and resonance shifts are discussed. (C) 1998 Elsevi
er Science B.V. All rights reserved.