Thermally deposited ultrathin Fe films on Cu(111) at room temperature
or below have been known to grow in a multilayer mode with a low net m
agnetic moment (similar to 0.5 mu(B)). In the present work we have use
d pulsed laser deposition to produce isotropic fee Fe/Cu(111) films wh
ich grow layer by layer with a magnetic moment of more than 2 mu(B). W
e attribute the larger magnetic moment of the pulsed laser deposited f
ilms to their structural perfection as seen by low energy electron dif
fraction and scanning tunneling microscopy. [S0031-9007(98)05386-1].