T. Nikuni et Ae. Jacobs, QUANTUM FLUCTUATIONS IN THE INCOMMENSURATE PHASE OF CSCUCL3 IN A TRANSVERSE MAGNETIC-FIELD, Physical review. B, Condensed matter, 57(9), 1998, pp. 5205-5212
In zero magnetic field, the stacked, triangular antiferromagnet CsCuCl
3 has a helical structure incommensurate (IC) in the chain direction (
normal to the planes). A magnetic field applied transverse to the chai
ns distorts the helix, but the IC structure persists up to at least 0.
43 times the saturation field. The IC wave number q (from neutron-diff
raction experiments) decreases with increasing field, but then it has
an unexpected plateau. Classical theory explains the behavior at small
fields, including the temperature dependence, but it fails to explain
the plateau, which we ascribe to quantum fluctuations. We find that l
inear spin-wave (LSW) theory also fails to explain the plateau; in fac
t, LSW theory fails more severely than classical theory in describing
the IC phase. We introduce a phenomenological treatment of quantum flu
ctuations. After verifying that it describes well some known results,
we apply the phenomenological theory to the IC phase of CsCuCl3, findi
ng that it yields a plateau at approximately the observed value of q a
nd the observed fields; in addition, it predicts a transition to the c
ommensurate phase so far not observed. Results depend sensitively on a
weak anisotropy: A deviation of less than 1% from isotropy in the int
rachain ferromagnetic exchange changes the phase diagram completely at
fields above about half the saturation value.