Suspensions comprised of neutrally buoyant spheres in Newtonian fluids
undergoing creeping flow in the annular region between two rotating,
coaxial cylinders (a wide-gap Couette) display a bulk migration of par
ticles towards regions of lower shear rate. A series of experiments ar
e performed to characterize this particle migration, including the inf
luence of particle size, surface roughness, and volume fraction. Littl
e, if any, effect of particle surface roughness is observed. An existi
ng continuum diffusive-flux model [Phillips et ni. (1992)] for predict
ing particle concentration profiles in monomodal suspensions is evalua
ted using the current series of experimental data. This model predicts
a dependence of the migration rate on the square of the suspended par
ticles' radius, a(2). whereas the present experiments indicate that sy
stems with average particle volume fractions of 50% display a rate tha
t scales with a(3). Previous use of the diffusive-flux model has assum
ed constant values far diffusion coefficients which serve as tuning pa
rameters in the phenomenological equation. Here the experimental data
are used to investigate variations of the model in which the diffusion
coefficients depend upon either the local or global particle volume f
raction. For initially uniform suspensions, the coefficients are found
to be best modeled as functions of the local particle volume fraction
. (C) 1998 The Society of Rheology. [S0148-6055(98)01002-5].