The infrared spectrum of single oxygen carbon sulfide (OCS) molecules
was measured inside large superfluid pure helium-4 droplets and nonsup
erfluid pure helium-3 droplets, both consisting of about 10(4) atoms.
In the helium-4 droplets, sharp rotational lines were observed, wherea
s in helium-3 only a broad peak was found. This difference is interpre
ted as evidence that the narrow rotational lines, which imply free rot
ations, are a microscopic manifestation of superfluidity. Upon additio
n of 60 helium-4 atoms to the pure helium-3 droplets, the same sharp r
otational lines were found; it appears that 60 is the minimum number n
eeded for superfluidity.