S. Tomic et al., LOW-FREQUENCY DIELECTRIC RESPONSE OF CHARGE-DENSITY-WAVE PINNED BY COMMENSURABILITY IN (2,5(OCH3)(2)DCNQI)(2)LI, Europhysics letters, 38(3), 1997, pp. 219-224
We have used complex conductivity measurements between 20 Hz and 1 MHz
to probe the dielectric response in the low-temperature phase of the
(2, 5(OCH3)(2)DCNQI)(2)Li organic conductor. The observed data reveal
the existence of the relaxation process which is well described by a D
ebye-like expression for an overdamped response of a system with a sin
gle degree of freedom. Both the static dielectric constant (epsilon(0)
= 3 x 10(7)) and the characteristic relaxation time (tau(0)) are much
larger than that expected for single-particle excitations. tau(0) is
thermally activated in a manner similar to the de conductivity. We att
ribute the observed relaxation to N = 4 charge density wave pinned by
commensurability to the underlying lattice.