R. Akimoto et al., LARMOR PRECESSION OF MN2+ MOMENTS INITIATED BY THE EXCHANGE FIELD OF PHOTOINJECTED CARRIERS IN CDTE CD1-XMNXTE QUANTUM-WELLS/, Physical review. B, Condensed matter, 57(12), 1998, pp. 7208-7213
We observed dynamical processes of the magnetic moments of photoinject
ed carriers and resultant perturbed magnetic moment of Mn2+ ions in Cd
Te/Cd1-xMnxTe quantum wells by means of the femtosecond time-resolved
magneto-optical Kerr rotation measurement in transverse magnetic field
s. The time-resolved Kerr rotation signal shows that the Larmor preces
sion of Mn2+ moment is initiated by photoinjected carriers. In particu
lar, we observed a time delay in terms of the phase and an amplitude o
f Mn2+ beats as a function of the external field to confirm the mechan
ism of perturbing the Mn2+ moment, i.e., a transient p-d exchange fiel
d, proposed in earlier studies. The motion of the Mn2+ moment is also
simulated by the Bloch model including the impulsive transverse exchan
ge fields produced by the conduction electron and heavy-hole spins. Fr
om this it is found that the exchange field of the heavy-hole spin con
tributes dominantly to tipping the Mn2+ moment away from the external
field axis. The exchange field estimated by the Bloch model so as to f
it experimental data is in reasonable agreement with the exchange fiel
d estimated from p-d exchange interaction, which also supports the abo
ve mechanism.