Superdeformation studies in Tl-189,Tl-191,Tl-192 Gammasphere are discu
ssed. New results on Tl-191 are the observation of interband transitio
ns between the signature partner E2 bands and the measurement of an av
erage quadrupole moment (Q(0) = 18 +/- eb) for these superdeformed str
uctures. These data enable us to derive absolute M1 strengths and conf
irm that the 81(st) proton occupies the [642]5/2 orbital. Tentative da
ta for one superdeformed sequence in Tl-189 are consistent with the pr
ediction of a decrease in quadrupole deformation for the lightest nucl
ei at the limit of this island of superdeformation.