We have developed a complete infrared absorption and tomographic inver
sion system. The source, a computer-controlled KCl:Li color center las
er, is tunable over the 2.45-2.82 mu m range, allowing spectral access
to many combustion and incineration products. A fast wavelength-locki
ng algorithm, in conjunction with the laser linewidth of similar to 0.
1 cm(-1), ensures line-center measurements for determination of temper
ature and concentration. The newly developed tomographic inversion met
hod takes maximum advantage of a priori information, and can require o
nly a small number of well-configured line-of-sight measurements to pr
oduce accurate reconstructions. Numerical experiments using simulated
absorption data to reconstruct both temperature and concentration dist
ributions have been performed. As few as 20 line-of-sight measurements
are required to produce high-fidelity reconstructions in these numeri
cal experiments.