Polycrystalline CrO2 is shown to exhibit a giant magnetoresistance (GM
R) at low temperatures. A rapid decrease in the GMR with increasing te
mperature is correlated with a decrease in the intergranular resistanc
e. Single-crystal CrO2 is a half-metallic ferromagnet, as the data are
interpreted to reflect two types of charge carriers, crossing a grain
boundary: those that tunnel between conduction bands of adjacent grai
ns and those that hop after residing at a localized state fora time lo
ng compared to a spin relaxation time. (C) 1998 American Institute of
Physics.