SPIN-PEIERLS GAP AND 2-MAGNETIC-EXCITATION BOUND AND RESONANT STATES IN CU1-XZNXGEO3 AND CUGE1-YSIYO3

Citation
T. Sekine et al., SPIN-PEIERLS GAP AND 2-MAGNETIC-EXCITATION BOUND AND RESONANT STATES IN CU1-XZNXGEO3 AND CUGE1-YSIYO3, Journal of the Physical Society of Japan, 67(4), 1998, pp. 1440-1450
Citations number
49
Categorie Soggetti
Physics
ISSN journal
00319015
Volume
67
Issue
4
Year of publication
1998
Pages
1440 - 1450
Database
ISI
SICI code
0031-9015(1998)67:4<1440:SGA2BA>2.0.ZU;2-C
Abstract
We study a spin-Peierls gap and a bound and a resonant states of two m agnetic excitations in Cu1-xZnxGeO3 and CuGe1-ySiyO3. Breakdown of the selection rule in the doped samples enables us to observe the spin-Pe ierls gap excitation in the first-order Raman process. It is found tha t this excitation shifts to lower frequency and merges into the tail o f the elastic scattering together with its line broadening with increa sing dopant concentration. The bound state of a particle-hole pair is observed just below the bottom of the second-order Raman band in pure CuGeO3. It changes into a resonant state and disappears rapidly as the concentration of the dopant is increased, owing to the weakening of a ttractive interaction and the extreme increase of the dampings of the magnetic excitations. These features are demonstrated theoretically by using Green's function.