T. Riste et K. Otnes, OBSERVATION OF FLUCTUATIONS IN A 3-DIMENSIONAL HEISENBERG-SYSTEM WITHPOSITIONAL DISORDER, Physica. B, Condensed matter, 213, 1995, pp. 152-154
Several years ago de Gennes predicted that orientational director fluc
tuations in a nematic liquid crystal, in zero field, fulfill the condi
tions of a 3D Heisenberg system. The verification of this prediction b
y neutron scattering represents a challenge, since the relevant time s
cale is macroscopic and the substance has no positional order. We have
looked for real-time fluctuations of the liquid diffraction peaks and
analyzed the observed time series by the Hurst-exponent (H) method. I
n zero magnetic field we find H similar to 1, indicating infinite temp
oral correlations between orientational fluctuations of the director.
With increasing magnetic field we observe a cross-over to H similar to
0.5, corresponding to zero temporal correlations. A similar cross-ove
r is found by the application of a temperature gradient, or by heating
to the isotropic liquid phase.