Sn. Orlov et Yn. Polivanov, ELIMINATION OF THE BACKGROUND FROM POLARITON CARS SPECTRA BY SPATIAL SEPARATION OF THE EXCITING AND PROBE BEAMS, Quantum electronics, 28(2), 1998, pp. 167-168
A method for elimination of the background (resulting from direct four
-photon processes) from polariton CARS spectra is proposed and demonst
rated experimentally. The method is based on the ability of polaritons
to propagate in a medium over macroscopic distances and it requires a
geometry of the interacting waves in which the regions of biharmonic
excitation of polaritons and probing of the excited polaritons by a pr
obe beam are spatially separated in a crystal.