J. Ishi et al., 3RD-ORDER OPTICAL NONLINEARITY DUE TO EXCITONS AND BIEXCITONS IN A SELF-ORGANIZED QUANTUM-WELL MATERIAL (C6H13NH3)(2)PBI4, Journal of nonlinear optical physics and materials, 7(1), 1998, pp. 153-159
Third-order optical nonlinearity around the exciton resonance in (C6H1
3NH3)(2)PbI4 was measured using time-integrated and spectrally-resolve
d four-wave-mixing (FWM) techniques. For excitation below the exciton
resonance, biexciton contribution to the FWM signals was observed. The
dephasing energy of the biexcitons was estimated to be larger than 10
meV.