MOLECULAR-DYNAMICS STUDY OF LONG-LIVED STRUCTURES IN A FRAGILE GLASS-FORMING LIQUID

Citation
G. Johnson et al., MOLECULAR-DYNAMICS STUDY OF LONG-LIVED STRUCTURES IN A FRAGILE GLASS-FORMING LIQUID, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 57(5), 1998, pp. 5707-5718
Citations number
50
Categorie Soggetti
Physycs, Mathematical","Phsycs, Fluid & Plasmas
ISSN journal
1063651X
Volume
57
Issue
5
Year of publication
1998
Part
B
Pages
5707 - 5718
Database
ISI
SICI code
1063-651X(1998)57:5<5707:MSOLSI>2.0.ZU;2-7
Abstract
We present molecular-dynamics results for a two-component, two-dimensi onal Lennard-Jones supercooled liquid near the glass transition. We fi nd that the supercooled liquid is spatially heterogeneous and that the re are long-lived clusters whose size distribution satisfies a scaling relation up to a cutoff. The similarity of several properties of the supercooled liquid to those of a mean-field glass-forming fluid near t he spinodal suggests that the glass transition in the supercooled liqu id is associated with an underlying thermodynamic instability.