G. Johnson et al., MOLECULAR-DYNAMICS STUDY OF LONG-LIVED STRUCTURES IN A FRAGILE GLASS-FORMING LIQUID, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 57(5), 1998, pp. 5707-5718
We present molecular-dynamics results for a two-component, two-dimensi
onal Lennard-Jones supercooled liquid near the glass transition. We fi
nd that the supercooled liquid is spatially heterogeneous and that the
re are long-lived clusters whose size distribution satisfies a scaling
relation up to a cutoff. The similarity of several properties of the
supercooled liquid to those of a mean-field glass-forming fluid near t
he spinodal suggests that the glass transition in the supercooled liqu
id is associated with an underlying thermodynamic instability.