N. Balakrishnan et al., TIME-DEPENDENT QUANTUM-MECHANICAL APPROACH TO REACTIVE SCATTERING ANDRELATED PROCESSES, Physics reports, 280(2), 1997, pp. 80-144
The time-dependent quantum mechanical approach has emerged as a powerf
ul and a practical computational tool for studying a variety of gas-ph
ase chemical problems in recent years. In this report, we discuss the
various developments that have made this possible with special emphasi
s on methodology and application to reactive scattering, photo-excitat
ion processes and gas-surface interaction.