A. Tobo et al., EXCESS MAGNETIZATION OF THE DILUTED ANTIFERROMAGNET MNXMG1-XTIO3 IN LOW FIELDS, Journal of the Physical Society of Japan, 67(5), 1998, pp. 1784-1790
The temperature dependence of the excess magnetization Delta M = M-FC
- M-ZFC at low fields is examined for the diluted antiferromagnet MnxM
g1-xTiO3 with x greater than or equal to 0.62. The Delta M appears at
a temperature a little higher than the respective Neel temperature; an
d it increases as the temperature decreases. Except the difference of
the scale factor, the shape of Delta M vs T curves does not depend on
the applied magnetic fields and the magnetic ion concentrations at low
fields for the x greater than or equal to 0.64 samples. Moreover, we
have firstly found that the temperature dependence of Delta M coincide
s with that of the squared sublattice magnetization. The shape of Delt
a M vs T curves is also similar to those of the other several diluted
antiferromagnets with weak anisotropy reported for the low field regio
n. We show that the appearance of Delta M does not originate directly
from the random-field effect. The origin of Delta M is discussed.