M. Mauro et I. Oppenheim, Microscopic theory for hopping transport in glass-forming liquids: mode coupling corrections, PHYSICA A, 265(3-4), 1999, pp. 520-534
By introducing an order parameter that describes the geometry of clusters o
f particles, Liu and Oppenheim [Physica A 247 (1997) 183] developed a micro
scopic theory for hopping transport in glass-forming liquids. In this work
we bring this theory within the frame of mode coupling theories in the high
ly viscous regime. We calculate corrections to the effective longitudinal v
iscosity that affect its long-time dynamical behavior. Nevertheless, the re
lation between the longitudinal viscosity and the hopping kernel is not qua
litatively altered by mode coupling. (C) 1999 Elsevier Science B.V. All rig
hts reserved.