The early stages of homoepitaxy on the GaAs (001)-(2 x 4) surface have been
studied by scanning tunnelling microscopy (STM). Detailed island statistic
s have been obtained from STM images and show a clear dependence on both th
e arsenic species used and the incident arsenic flux. These results are exp
lained by considering the effects of the macroscopic arsenic kinetics (As-2
and As-4) on island nucleation and growth at the nanometre scale. (C) 1999
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