Femtosecond mid-infrared laser pulses that are continuously tunable in
the wavelength range from 9 to 18 mu m are demonstrated. These nearly
bandwidth-limited pulses are generated by phase-matched difference-fr
equency mixing within the broad spectrum of 20-fs pulses from a mode-l
ocked Ti:sapphire laser in GaSe. A direct determination of the pulse d
uration at 11.5 mu m gives a value of 140 fs. The average mid-infrared
power of 1 mu W is similar to 100 times greater than that for infrare
d generation by non-phase-matched optical rectification. (C) 1998 Opti
cal Society of America.