T. Muranaka et Y. Hiwatari, SPATIAL HETEROGENEITY IN SUPERCOOLED LIQUIDS AND GLASSES, Journal of the Physical Society of Japan, 67(6), 1998, pp. 1982-1987
The dynamical properties of the supercooled liquids and glasses have b
een studied via molecular dynamics (MD) simulation. We have found the
spatial heterogeneity for long time region in our model fluids. The ma
in factor of this heterogeneity originates from the linearly correlate
d jump motion, which changes the configurations even in the glass stat
e. This type of jump motion is assisted by the linearly correlated mot
ion which takes place in much shorter time region than that of the res
idence time of successive jump motions. Therefore it is concluded that
the longtime heterogeneity in glasses originates from the linearly co
rrelated motion in short time region.