SPATIAL HETEROGENEITY IN SUPERCOOLED LIQUIDS AND GLASSES

Citation
T. Muranaka et Y. Hiwatari, SPATIAL HETEROGENEITY IN SUPERCOOLED LIQUIDS AND GLASSES, Journal of the Physical Society of Japan, 67(6), 1998, pp. 1982-1987
Citations number
34
Categorie Soggetti
Physics
ISSN journal
00319015
Volume
67
Issue
6
Year of publication
1998
Pages
1982 - 1987
Database
ISI
SICI code
0031-9015(1998)67:6<1982:SHISLA>2.0.ZU;2-#
Abstract
The dynamical properties of the supercooled liquids and glasses have b een studied via molecular dynamics (MD) simulation. We have found the spatial heterogeneity for long time region in our model fluids. The ma in factor of this heterogeneity originates from the linearly correlate d jump motion, which changes the configurations even in the glass stat e. This type of jump motion is assisted by the linearly correlated mot ion which takes place in much shorter time region than that of the res idence time of successive jump motions. Therefore it is concluded that the longtime heterogeneity in glasses originates from the linearly co rrelated motion in short time region.