The formation of multiple nuclear spin echo signals has been studied i
n thin ferromagnetic polycrystalline films of 3d-metals and their allo
ys with induced anisotropy at temperatures between 2.2 and 300 K using
two-pulse and three-pulse excitation. A method is proposed for the ex
perimental determination of the contributions made by different mechan
isms to the formation of spin-echo signals in magnets with strongly in
homogeneous Zeeman and quadrupole interactions, It is shown that in fe
rromagnets with a high rf field gain at the nucleus, the frequency mod
ulation mechanism has a substantial influence in observations of nucle
ar spin-echo signals at nuclei with a high magnetic moment, even at li
quid-helium temperatures. (C) 1998 American Institute of Physics.