ON-SITE COULOMB REPULSION IN THE SMALL POLARON SYSTEM LA1-XCAXMNO3

Citation
Dc. Worledge et al., ON-SITE COULOMB REPULSION IN THE SMALL POLARON SYSTEM LA1-XCAXMNO3, Physical review. B, Condensed matter, 57(24), 1998, pp. 15267-15271
Citations number
31
Categorie Soggetti
Physics, Condensed Matter
ISSN journal
01631829
Volume
57
Issue
24
Year of publication
1998
Pages
15267 - 15271
Database
ISI
SICI code
0163-1829(1998)57:24<15267:OCRITS>2.0.ZU;2-G
Abstract
Conductivity measurements from 300 to 1200 K of La1-xCaxMnO3 thin film s, with doping from x=0 to x=1, show that the entire doping range fits the adiabatic small polaron model sigma=(A/T)exp(-E-a/kT). Furthermor e the x dependence of A explicitly shows the effects of on-site Coulom b repulsion, i.e., a polaron cannot hop into an occupied site. Instead of increasing monotonically as more carriers are introduced, A starts to decrease at x=0.2 and, as expected for Hubbard band splitting, is reduced to almost zero when the lattice is full.