On the basis of the International Atomic Energy Agency/World Meteorolo
gical Organization (IAEA\WMO) data set of the monthly tritium concentr
ation in precipitation, the temporal and spatial pattern of the tritiu
m concentration in marine precipitation of the southern hemisphere has
been reconstructed. A numerical model that couples the tritium concen
trations in the atmosphere and in the Weddell Sea's surface layer by p
arameterizing the relevant flux and exchange mechanisms, as well as th
e surface layer dynamics, has been used to calculate the time history
of tritium in near-surface waters of the Weddell Sea, The model also s
imulates the gas transfer of the chlorofluorocarbons CFC 11 and CFC 12
and of helium across the ocean-atmosphere interface. The model accoun
ts for the pronounced seasonality of the climatological and oceanograp
hic conditions of the Weddell Sea. The calculated input functions of t
ritium, CFC 11 and CFC 12 provide the surface boundary conditions for
numerical studies of the distributions of these transient tracers in t
he sub-surface water masses of the Weddell Sea.