Mission 12 of the first Aerosol Characterization Experiment was flown
by the National Center for Atmospheric Research C-130 research aircraf
t to observe stratocumulus cloud decks over the remote Southern Ocean.
The objective of the flight was the investigation of the impact of cl
ouds on the formation and destruction of aerosol in the boundary layer
. The principle focus of this paper is an examination of the thermodyn
amic structure and a quantification of the entrainment rate. Three met
hods are presented. The first method uses the thermodynamic budget of
the boundary layer to calculate its evolution over time. The second us
es turbulence flux observations near the inversion, while the third us
es estimates of the subsidence rate together with direct observations
of the rate of change of cloud top height. All three methods suffer fr
om serious errors. Our best estimate for the entrainment rate is 4 mm
s(-1) with an uncertainty of at least 50%. Based on an analysis of the
boundary layer evolution in a mixing diagram, entrainment rates large
r than about 8 mm s(-1) can probably excluded because these larger ent
rainment rates would impose an unrealistic thinning of the cloud layer
. Similarly, entrainment rates smaller than 2 mm s(-1) can be excluded
as well on the basis that this would impose unrealistic thickening of
the cloud layer. The boundary layer is mostly buoyancy-driven, with s
hear-generated turbulence at most only half of the buoyancy-generated
turbulence.