ENERGY RELAXATION DURING THERMALLY ACTIVATED DIFFUSION ALONG ONE-DIMENSIONAL CHAINS WITH SITE DISORDER

Citation
Ya. Berlin et Lda. Siebbeles, ENERGY RELAXATION DURING THERMALLY ACTIVATED DIFFUSION ALONG ONE-DIMENSIONAL CHAINS WITH SITE DISORDER, Chemical physics letters, 291(1-2), 1998, pp. 85-93
Citations number
32
Categorie Soggetti
Physics, Atomic, Molecular & Chemical
Journal title
ISSN journal
00092614
Volume
291
Issue
1-2
Year of publication
1998
Pages
85 - 93
Database
ISI
SICI code
0009-2614(1998)291:1-2<85:ERDTAD>2.0.ZU;2-P
Abstract
The energy relaxation during thermally activated diffusion along one-d imensional chains with equally spaced traps of random energy depths ha s been studied both analytically and by computer simulations. Several time intervals, where the mean particle energy exhibits distinct tempo ral and temperature behaviors, have been identified. The explicit form s of these dependencies within each of the intervals are specified. Th e results show that the relaxation of the mean particle energy and the time evolution of the average barrier height, probed by diffusing par ticles, follow a logarithmic law rather than the Kohlrausch-Williams-W att phenomenology. (C) 1998 Elsevier Science B.V. All rights reserved.