S. Guerin et Hr. Jauslin, 2-LASER MULTIPHOTON ADIABATIC PASSAGE IN THE FRAME OF THE FLOQUET THEORY - APPLICATIONS TO (1-STIRAP AND (2+1)-STIRAP(1)), EUROPEAN PHYSICAL JOURNAL D, 2(2), 1998, pp. 99-113
We develop an adiabatic two-mode Floquet theory to analyse multiphoton
coherent population transfer in Ai-level systems by two delayed laser
pulses, which is a generalization of the three-state stimulated Raman
adiabatic passage (STIRAP). The main point is that, under conditions
of non-crossing and adiabaticity, the outcome and feasibility of a STI
RAP process can be determined by the analysis of two features: (i) the
liking of degeneracy of dressed states at the beginning and at the en
d of the laser pulses, and (ii) the connectivity of these degeneracy-l
ifted branches in the quasienergy diagram. Both features can be determ
ined by stationnary perturbation theory in the Floquet representation.
As an illustration, we study the corrections to the RWA of the (1+1)
STIRAP in strong fields and for large detunings. We analyse the possib
le breakdown of connectivity. In strong fields, the complete transfer
is achieved, but the intermediate state, unpopulated within the RWA, c
an become populated during the process. In the (2+1) STIRAP, we show a
residual degeneracy in a four-level system, that can be liked by addi
tional Stark shifts. The complete transfer is achieved under condition
s of connectivity.