The present work establishes a methodology used to conduct a comparati
ve study of various probability distributions generally used to descri
be liquid spray atomization data. This methodology involves model disc
rimination and criticism, as well as random sampling used to obtain ob
jective criteria for choosing among rival models. Examples, representi
ng different atomization mechanisms, are given for the determination o
f the relative posterior probabilities of candidate models and for the
ir goodness of fit when models are fitted to a common data set. The me
thodology has been extended to include unreplicated data in addition t
o replicated data. The end result Is presented in a form suitable for
formulating empirical models of spray size distributions, with the int
ent of incorporating such models into multidimensional, two-phase flow
simulations.