We obtain femtosecond (200 fs) time resolution using a scanning tunnel
ing microscope on surface plasmon polaritons (SPPs) generated by two 1
00 fs laser beams in total internal reflection geometry. The tunneling
gap dependence of the signal clearly indicates the tunneling origin o
f the signal and suggests that nanometer spatial resolution can be obt
ained together with femtosecond temporal resolution. This fast respons
e, in contrast to the picosecond decay time of SPPs revealed by differ
ential reflectivity measurements, can be attributed to a coherent supe
rposition of SPPs rectified at the tunneling junction. (C) 1998 Americ
an Institute of Physics. [S0003-6951(98)02223-2].