This article presents a new method for determining particle size distr
ibution in undiluted suspensions from spectral measurement of transpor
t-scattering coefficients using continuous-wave photon migration techn
iques. Particle size distribution (PSD) for concentrated suspensions i
s determined by a regularized inverse algorithm which makes it possibl
e to incorporate a synthesized scheme of Marquardt and Tikhonov regula
rizations. Spectral measurements of dense TiO2 suspensions with three
different particle concentrations were used to recover the suspensions
' size distributions. Our results are in excellent agreement with the
size distribution measured with X-ray sedimentation. These reconstruct
ions of PSDs are obtained both with and without a priori distribution
function assumptions.