RESONANT DOUBLE MULTIPHOTON IONIZATION VIA PLANETARY STATES

Citation
S. Cohen et al., RESONANT DOUBLE MULTIPHOTON IONIZATION VIA PLANETARY STATES, Journal of physics. B, Atomic molecular and optical physics, 26(21), 1993, pp. 3783-3794
Citations number
25
Categorie Soggetti
Physics, Atomic, Molecular & Chemical",Optics
ISSN journal
09534075
Volume
26
Issue
21
Year of publication
1993
Pages
3783 - 3794
Database
ISI
SICI code
0953-4075(1993)26:21<3783:RDMIVP>2.0.ZU;2-0
Abstract
We have studied double ionization of Ba 6snl Rydberg states through re sonant two-photon excitation of 8snl double-Rydberg states with n = 13 and 14 and different l. The laser intensity dependence of Ba2+ yield measured for / greater-than-equal-to 8, when the electrons suffer long -range dipole interaction, shows a decrease from four-photon for l = 8 to less than three for l = 11. The four-photon dependence is due to a utoionization decay populating the Ba+(7p) levels which gives an indir ect signature to the Ba2+ production. By increasing l this decay vanis hes and the data show evidence of a direct double-ionization process v ia planetary-electron states for l greater-than-or-equal-to 10. Additi onal intensity measurements performed for low l = 6 states strongly mi xed with 5fn'l' ones by short-range multipole interaction, reveal indi rect Ba2+ production and an individual case of partial stabilization d ue to destructive interference leading to direct double ionization.