Wt. Coffey et al., EFFECT OF AN OBLIQUE MAGNETIC FIELD ON THE SUPERPARAMAGNETIC RELAXATION-TIME - 2 - INFLUENCE OF THE GYROMAGNETIC TERM, Physical review. B, Condensed matter, 58(6), 1998, pp. 3249-3266
The effect of a uniform magnetic field applied at an oblique angle to
the easy axis of magnetization on the superparamagnetic (longitudinal
or Neel) re:laxation time is investigated by numerically solving the F
okker-Planck equation for the smallest nonvanishing eigenvalue. It is
demonstrated that the reciprocal of the asymptotic formula for the Kra
mers escape rate in the intermediate to high damping limit for general
nonaxially symmetric potentials when applied to the present problem,
yields an acceptable asymptotic approximation to the Neel time for mod
erate to high values of the damping. Alternatively the corresponding K
ramers low dissipation formula (energy controlled diffusion) provides
an acceptable approximation for very small values of the damping. The
effect of the gyromagnetic term which gives rise to coupling between t
he longitudinal and transverse modes of motion generally corresponds t
o an increase of the smallest nonvanishing eigenvalue and so to a decr
ease of the Neel relaxation time. The integral relaxation time or area
under the slope of the curve of the decay of the magnetization is als
o evaluated. It is demonstrated that for sufficiently high values-of t
he uniform field (much less, however, than that required to destroy th
e bistable nature of the potential) the reciprocal of the lowest nonva
nishing eigenvalue (proportional to the Neel time, or the time of reve
rsal of the magnetization) and the integral relaxation time may differ
exponentially from one another signifying the contributions of modes
other than that associated with the overbarrier (Neel) relaxation proc
ess to the overall relaxation process. The overall behavior is qualita
tively similar (apart from the azimuthal dependence) to that of the ax
ially symmetric case which arises due to the depletion of the shallowe
r of the two potential wells by the uniform field, so that the fast pr
ocesses in the deeper of the two wells may come to dominate the relaxa
tion process at sufficiently high values of the uniform field.