Single-bubble sonoluminescence has been experimentally produced throug
h a novel approach of optimized sound excitation. A driving consisting
of a first and second harmonic with selected amplitudes and relative
phase results in an increase of light emission compared to sinusoidal
driving. We achieved a raise of the maximum photocurrent of up to 300%
with the two-mode sound signal. Numerical simulations of multimode ex
citation of a single bubble are compared to this result.