Jh. Yi et al., THE EFFECT OF LASER-PULSE WIDTH ON THE MULTIPHOTON IONIZATION EFFICIENCY, Journal of the Korean Physical Society, 33(3), 1998, pp. 345-349
We studied the variation of the multi-photon ionization efficiencies o
f atoms as a function of the laser pulse width under the condition of
constant pulse energy. The density-matrix calculation showed that long
pulses were preferred for efficient ionization whenever the lifetimes
of the levels involved in the transition were longer than the pulse w
idths. Also, it was demonstrated that the atomic and the laser paramet
ers, such as transition cross-sections, laser pulse widths, and lifeti
mes affect the optimal excitation rate of the transition for efficient
multi-photon ionization.